early 15c., "too large to be conceived, unimaginable," from un- (1) "not" + think (v.) + -able. Meaning "incapable of being framed by thought" is recorded from mid-15c.
Entries linking to unthinkable
un- 1
prefix of negation, Old English un-, from Proto-Germanic *un- (source also of Old Saxon, Old Frisian, Old High German, German un-, Gothic un-, Dutch on-), from PIE *n- (source of Sanskrit a-, an- "not," Greek a-, an-, Old Irish an-, Latin in-), combining form of PIE root *ne- "not." Often euphemistic (such as untruth for "lie").
The most prolific of English prefixes, freely and widely used in Old English, where it forms more than 1,000 compounds. It underwent a mass extinction in early Middle English, but emerged with renewed vigor 16c. to form compounds with native and imported words. It disputes with Latin-derived cognate in- (1) the right to form the negation of certain words (indigestable/undigestable, etc.), and though both might be deployed in cooperation to indicate shades of meaning (unfamous/infamous), typically they are not.
It also makes words from phrases (such as uncalled-for, c. 1600; undreamed-of, 1630s; uncome-at-able, 1690s; unputdownable, 1947, of a book; un-in-one-breath-utterable, Ben Jonson; etc., but the habit is not restricted to un-; such as put-up-able-with, 1812). As a prefix in telegramese to replace not and save the cost of a word, it is attested by 1936.
think v.
Old English þencan "imagine, conceive in the mind; consider, meditate, remember; intend, wish, desire" (past tense þohte, past participle geþoht), probably originally "cause to appear to oneself," from Proto-Germanic *thankjan (source also of Old Frisian thinka, Old Saxon thenkian, Old High German denchen, German denken, Old Norse þekkja, Gothic þagkjan).
Old English þencan is the causative form of the distinct Old English verb þyncan "to seem, to appear" (past tense þuhte, past participle geþuht), from Proto-Germanic *thunkjan (source also of German dünken, däuchte). Both are from PIE *tong- "to think, feel" which also is the root of thought and thank.
The two Old English words converged in Middle English and þyncan "to seem" was absorbed, except for its preservation in archaic methinks "it seems to me."
As a noun, think, "act of prolonged thinking," is attested by 1834. The figurative thinking cap is attested from 1839.