Old English uncynde "unnatural, not natural;" see un- (1) "not" + kind (adj.). Meaning "lacking in kindness" is recorded from mid-14c.
Entries linking to unkind
un- 1
prefix of negation, Old English un-, from Proto-Germanic *un- (source also of Old Saxon, Old Frisian, Old High German, German un-, Gothic un-, Dutch on-), from PIE *n- (source of Sanskrit a-, an- "not," Greek a-, an-, Old Irish an-, Latin in-), combining form of PIE root *ne- "not." Often euphemistic (such as untruth for "lie").
The most prolific of English prefixes, freely and widely used in Old English, where it forms more than 1,000 compounds. It underwent a mass extinction in early Middle English, but emerged with renewed vigor 16c. to form compounds with native and imported words. It disputes with Latin-derived cognate in- (1) the right to form the negation of certain words (indigestable/undigestable, etc.), and though both might be deployed in cooperation to indicate shades of meaning (unfamous/infamous), typically they are not.
It also makes words from phrases (such as uncalled-for, c. 1600; undreamed-of, 1630s; uncome-at-able, 1690s; unputdownable, 1947, of a book; un-in-one-breath-utterable, Ben Jonson; etc., but the habit is not restricted to un-; such as put-up-able-with, 1812). As a prefix in telegramese to replace not and save the cost of a word, it is attested by 1936.
kind adj.
"friendly, deliberately doing good to others," Middle English kinde, from Old English (ge)cynde "natural, native, innate," originally "with the feeling of relatives for each other," from Proto-Germanic *kundi- "natural, native," from *kunjam "family" (see kin), with collective or generalizing prefix *ga- and abstract suffix *-iz. The word rarely appeared in Old English without the prefix, but Old English also had it as a word-forming element -cund "born of, of a particular nature" (see kind (n.)). Sense development probably is from "with natural feelings," to "well-disposed" (c. 1300), "benign, compassionate, loving, full of tenderness" (c. 1300).
unkindness n.
c. 1300, "state or character of being unkind, lack of natural regard or proper consideration," from un- (1) "not" + kindness (n.), or from unkind (adj.) + -ness. Meaning "an unkind act" is from c. 1500.