mid-14c., "not possessed of book-learning," from un- (1) "not" + lettered. An Englished form of illiterate. Similar formation in Middle Dutch ongelettert.
Entries linking to unlettered
un- 1
prefix of negation, Old English un-, from Proto-Germanic *un- (source also of Old Saxon, Old Frisian, Old High German, German un-, Gothic un-, Dutch on-), from PIE *n- (source of Sanskrit a-, an- "not," Greek a-, an-, Old Irish an-, Latin in-), combining form of PIE root *ne- "not." Often euphemistic (such as untruth for "lie").
The most prolific of English prefixes, freely and widely used in Old English, where it forms more than 1,000 compounds. It underwent a mass extinction in early Middle English, but emerged with renewed vigor 16c. to form compounds with native and imported words. It disputes with Latin-derived cognate in- (1) the right to form the negation of certain words (indigestable/undigestable, etc.), and though both might be deployed in cooperation to indicate shades of meaning (unfamous/infamous), typically they are not.
It also makes words from phrases (such as uncalled-for, c. 1600; undreamed-of, 1630s; uncome-at-able, 1690s; unputdownable, 1947, of a book; un-in-one-breath-utterable, Ben Jonson; etc., but the habit is not restricted to un-; such as put-up-able-with, 1812). As a prefix in telegramese to replace not and save the cost of a word, it is attested by 1936.
lettered adj.
"literate, learned in letters," c. 1300, from letter (n.1). Meaning "inscribed" is from 1660s, from letter (v.).
illiterate adj.
early 15c., "uneducated, unable to read and write" (originally meaning Latin), from Latin illiteratus "unlearned, unlettered, ignorant; without culture, inelegant," from assimilated form of in- "not, opposite of" (see in- (1)) + literatus "educated," literally "furnished with letters" (see literate). Old English used unstæfwis as a loan-translation of Latin illiteratus. As a noun meaning "illiterate person" from 1620s. Hence, illiterati (1788, Horace Walpole).